Preprint: Towards a gigantic Magnus balloon with motorized belts

Or we are ignorant of the solutions that are already used. Hydrogen is the best option, if you explore the idea of lighter than air balloons you should look at hydrogen first and make sure that it is difficult to implement, and not just seems to be so. If hydrogen is difficult, any other solution is going to be either more difficult, or plain “impossible”.

So you add a hydrogen sensor. And IIRC you would always have an ignition source so the flame/explosion would occur as soon as possible, limiting the size of the explosion. That is if you are using hydrogen-filled ballonets inside the balloon leaking hydrogen into the balloon.

One idea might be to fill the balloon with nitrogen instead of or in addition to air, but I think then the risk of asphyxiation might exceed the original risk of explosion. Maybe there is a balance.

Using methane is your idea. Do the homework yourself. You can compare the cost of the gas, cost of the larger envelope, impact on other aspects of the design from the lower lift, and so on.